Yes, you can label the bar chart on or near the bar itself. In the Contents Pane, select the layer in question, then click Feature Layer->Symbology. Identify the field to label in the Label Class group and click Label in the Layer group. You can open the Label Class pane and set the properties of the label appearance using the Maplex Labeling Engine. See image below for my example.
Great! If you feel my answer is correct, you can close this thread by marking the response as the solution. Good luck with all things ArcGIS Pro - cheers!
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