I believe what you're referring to is Single-Sign-On (SSO). SSO for Windows Integrated Authentication will work with ArcGIS for Server but I believe your users and roles all need to come from the same provider. In other words, I don't think you can use a mixed configuration whereby users come from the domain and roles come from the built-in store as an example.
Hi William, I'm sorry to confuse you. I would like to secure services and expose them, over the internet, to users that do not have a user account in my network's windows active directory. I added them as a user in IIS, which provides them access to the web app, but what you're saying is that it's not possible to somehow pass the IIS windows log-in credentials to the secured services then, correct?
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